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| Date | Competition | Venue | Opponent | Programme | Notes | Aug 6 | Fr | H | Manchester City | | | Aug 13 | LC | H | St Johnstone | | | Aug 17 | LC | A | Dundee | | | Aug 20 | LC | H | Dundee United | | | Aug 27 | LC | A | St Johnstone | | | Aug 31 | LC | H | Dundee | | | Sep 3 | LC | A | Dundee United | | | Sep 10 | D1 | A | Dundee | | | Sep 14 | LC | A | Morton | | | Sep 17 | D1 | H | St Johnstone | | | Sep 21 | LC | H | Morton | | | Sep 24 | D1 | A | Rangers | Y | | Oct 1 | D1 | H | Clyde | Y | | Oct 5 | Fr | A | Deveronvale | | | Oct 8 | D1 | A | Dunfermline Athletic | | | Oct 15 | D1 | H | Ayr United | | | Oct 19 | LC | Hampden | Rangers | | | Oct 22 | D1 | A | Airdrie | | | Oct 24 | LC | Hampden | Rangers | N | | Oct 29 | D1 | H | Hibernian | | | Nov 5 | D1 | H | Hearts | | | Nov 12 | D1 | A | St Mirren | | | Nov 19 | D1 | H | Partick Thistle | | | Nov 26 | D1 | A | Dundee United | | | Dec 3 | D1 | H | Motherwell | | | Dec 10 | D1 | A | Falkirk | | | Dec 17 | D1 | A | Stirling Albion | Y | | Dec 24 | D1 | H | Celtic | | | Dec 31 | D1 | H | Kilmarnock | | | Jan 2 | D1 | h | Dundee | | | Jan 3 | D1 | A | St Johnstone | | | Jan 14 | D1 | A | Clyde | | | Jan 18 | D1 | H | Rangers | | | Jan 21 | D1 | H | Dunfermline Athletic | | | Jan 28 | SC | A | Dundee | | | Feb 4 | D1 | A | Ayr United | | | Feb 11 | D1 | H | Airdrie | | | Feb 18 | SC | H | St Johnstone | | | Feb 25 | D1 | A | Hibernian | | | Mar 4 | D1 | A | Hearts | | | Mar 11 | SC | A | Hibernian | Y | | Mar 18 | D1 | A | Partick Thistle | | | Mar 22 | SC | H | Hibernian | | | Mar 25 | D1 | H | Dundee United | | | Mar 27 | D1 | H | St Mirren | | | Apr 1 | SC | Dens Park | Dundee United | | | Apr 4 | D1 | A | Motherwell | | | Apr 8 | D1 | H | Falkirk | | | Apr 15 | D1 | H | Stirling Albion | | | Apr 19 | D1 | A | Celtic | | | Apr 29 | SC | Hampden | Celtic | | | May 1 | D1 | A | Kilmarnock | | | May 16 | Fr | A | Peterhead | | | May 18 | Fr | Woodside | Arbroath | | Lads Club Benefit match | May 27 | Fr | Washington | Stoke City | | USA Presidents Cup | May 31 | Fr | Toronto | Hibernian | | USA Presidents Cup | Jun 3 | Fr | Washington | Cagliari | | USA Presidents Cup | Jun 7 | Fr | Washington | Cerro | | USA Presidents Cup | Jun 11 | Fr | Detroit | Glentoran | | USA Presidents Cup | Jun 14 | Fr | Cleveland | Stoke City | | USA Presidents Cup | Jun 20 | Fr | Washington | Wolverhampton Wanderers | | USA Presidents Cup | Jun 25 | Fr | San Francisco | ADO Den Hague | | USA Presidents Cup | Jun 28 | Fr | Washington | Sunderland | | USA Presidents Cup | Jul 1 | Fr | Dallas | Dundee United | | USA Presidents Cup | Jul 4 | Fr | Houston | Bangu | | USA Presidents Cup | Jul 8 | Fr | Washington | Shamrock Rovers | | USA Presidents Cup | Jul 10 | Fr | Washington | Wolverhampton Wanderers | | USA Presidents Cup | Jul 14 | Fr | Los Angeles | Wolverhampton Wanderers | | USA Presidents Cup |
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|  Stirling Albion - D1 17 Dec 1966 | |  Rangers - D1 24 Sep 1966 | |
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